毫纳结构复合材料的制备、协同效应及其深度水处理应用

付宛宜; 李雨航; 杨志超; 张延扬; 张孝林; 刘子尧; 潘丙才

doi:10.7536/PC230510

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化学进展 ›› 2023, Vol. 35 ›› Issue (10) : 1415-1437. DOI: 10.7536/PC230510

综述

毫纳结构复合材料的制备、协同效应及其深度水处理应用

付宛宜 ¹ ,
李雨航 ¹ ,
杨志超 ¹ ,
张延扬 ¹^,² ,
张孝林 ¹^,² ,
刘子尧 ¹ ,
潘丙才 ¹^,²^,^*

作者信息 +

Millimeter-Sized Nanocomposites for Advanced Water Treatment: Preparation, Synergistic Effects and Applications

Wanyi Fu ¹ ,
Yuhang Li ¹ ,
Zhichao Yang ¹ ,
Yanyang Zhang ¹^,² ,
Xiaolin Zhang ¹^,² ,
Ziyao Liu ¹ ,
Bingcai Pan ¹^,²^,^*

Author information +

文章历史 +

摘要

纳米材料具有较高的比表面积和较强的表面效应,在水处理领域展现出优异的净污性能,具有广阔的应用前景。将纳米颗粒负载于毫米级载体中制备毫纳结构复合材料,可有机结合纳米颗粒的高反应活性与载体的良好操作性,是突破纳米材料易聚团失活、难分离、稳定性差、潜在环境风险等工程应用瓶颈并实现规模化应用的重要技术手段。本文综述了毫纳结构复合材料的制备方法、结构特性及其在吸附和催化氧化除污性能及机制方面的研究进展,并从纳米颗粒的限域生长、限域吸附特性和限域催化氧化特性等方面阐述限域效应及载体-纳米颗粒的协同净污效应。最后,针对目前毫纳结构复合材料方向亟待解决的科学问题和实际应用挑战提出了展望,以期为推动纳米材料的实际应用提供一定的理论指导和技术参考。

Abstract

Nanomaterial features a high surface area-to-volume ratio and strong surface effects, offering excellent performance in water treatment and broad application prospects. Incorporating nanoparticles into millimeter-scale hosts to prepare millimeter-sized nanocomposite materials can couple the high reactivity of nanoparticles with the easy operability of millimeter-scale hosts. This is an important technical approach to overcome the engineering application bottlenecks of nanomaterials, such as their tendency to agglomerate, low stability, potential environmental risks, and difficult separation. This review summarizes the preparation methods, structural characteristics, and adsorptive and catalytic oxidative removal of pollutants from aqueous systems by millimeter-sized nanocomposites. It elaborates on the confinement effects from the perspectives of confined growth of nanoparticles, confined adsorption properties, and confined catalytic oxidation properties, as well as the synergistic purification effect between the hosts and nanoparticles. Finally, the scientific issues and practical challenges that urgently need to be addressed in the development of millimeter-sized nanocomposites are discussed. We believe this review will provide theoretical guidance and technical references for promoting the practical applications of nanomaterials.

Contents

1 Introduction

2 Common hosts and preparation methods of millimeter-sized nanocomposites

2.1 Polymeric hosts

2.2 Carbon-based hosts

2.3 Natural mineral based hosts

2.4 Ceramic-based hosts

3 Confinement effects and synergistic purification effects of millimeter-nanometer structure

3.1 Confined growth of nanoparticles in millimeter-sized hosts

3.2 Confined adsorption and regeneration of nanoparticles inside millimeter-sized hosts

3.3 Confined catalytic oxidation of nanoparticles inside millimeter-sized hosts

4 Practical applications of millimeter-sized nanocomposites in water treatment

4.1 Applications in adsorption

4.2 Applications in catalytic degradation

5 Conclusions and perspectives

5.1 Research gaps in scientific issues regarding nanoconfinement effects

5.2 Challenges to be addressed for practical applications of nanocomposite materials

导出引用

付宛宜 , 李雨航 , 杨志超 , 等. 毫纳结构复合材料的制备、协同效应及其深度水处理应用[J]. 化学进展. 2023, 35(10): 1415-1437 https://doi.org/10.7536/PC230510

, , , et al. Millimeter-Sized Nanocomposites for Advanced Water Treatment: Preparation, Synergistic Effects and Applications[J]. Progress in Chemistry. 2023, 35(10): 1415-1437 https://doi.org/10.7536/PC230510

中图分类号： TB34 (功能材料) X703 (废水的处理与利用)

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基金

国家重点研发计划(2022YFA1205601)

国家重点研发计划(2022YFA1205602)

国家自然科学基金项目(21925602)

国家自然科学基金项目(22236003)

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收稿日期	修回日期	出版日期
2023-05-11	2023-06-10	2023-10-24
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2023-08-07

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