MIL-101(Fe) and Its Composites for Catalytic Removal of Pollutants: Synthesis Strategies, Performances and Mechanisms

Lan Mingyan; Zhang Xiuwu; Chu Hongyu; Wang Chongchen

doi:10.7536/PC220822

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Prog Chem ›› 2023, Vol. 35 ›› Issue (3) : 458-474. DOI: 10.7536/PC220822

Review

MIL-101(Fe) and Its Composites for Catalytic Removal of Pollutants: Synthesis Strategies, Performances and Mechanisms

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Abstract

MIL-101(Fe) is a typical Fe-based metal-organic framework (Fe-MOF), which demonstrates the advantages of flexible structure, large specific surface area, large porosity, and adjustable pore size. In recent years, MIL-101(Fe) and its composites have been extensively studied in the field of water pollution remediation, especially in the hexavalent chromium (Cr(Ⅵ)) reduction and advanced oxidation processes for removing organic pollutants in water. The water stability, light absorption activity and the carrier separation efficiency can be significantly improved by functional modification with specific functional materials. In this review, the preparation strategies of MIL-101(Fe) and its composites, as well as their application as heterogeneous catalysts for photocatalysis, H₂O₂ activation, and persulfate activation were introduced. The future development of MIL-101(Fe) and its composites as catalysts for water purification is prospected.

Key words

MIL-101(Fe) / catalysis / hexavalent chromium / organic pollutants / wastewater treatment

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Lan Mingyan , Zhang Xiuwu , Chu Hongyu , et al. MIL-101(Fe) and Its Composites for Catalytic Removal of Pollutants: Synthesis Strategies, Performances and Mechanisms[J]. Progress in Chemistry. 2023, 35(3): 458-474 https://doi.org/10.7536/PC220822

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Funding

National Natural Science Foundation of China(22176012)

Beijing Natural Science Foundation(8202016)

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2022-08-26	2023-01-08	2023-03-24
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