Condensed Matter Chemistry in Catalysis by Zeolites

Fengshou Xiao; Qinming Wu; Chengtao Wang

doi:10.7536/PC221008

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Prog Chem ›› 2023, Vol. 35 ›› Issue (6) : 886-903. DOI: 10.7536/PC221008

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Condensed Matter Chemistry in Catalysis by Zeolites

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Abstract

This work is devoted to condensed matter chemistry in gas-phase catalytic reactions over zeolite catalysts, which mainly involve in the processes of (i) adsorption of gaseous reactants into zeolite micropores, (ii) conversion of the reactants on catalytic sites in zeolites, and (iii) desorption of products in zeolites. In the above processes, both fast adsorption in zeolite micropores and rapid desorption from zeolites can significantly improve the reaction rate. To realize these purposes, it has been developed new strategies for rational synthesis of zeolites including preparation of zeolite nanocrystals, introduction of mesopores into zeolite crystals, preparation of zeolite nanosheets, and adjusting wettability of zeolite crystals, which have been simply concluded. Furthermore, the catalytically active sites including single atoms and metal nanoparticles can be introduced into zeolite frameworks or zeolite crystals, which can combine both the advantages of high stability and excellent shape selectivity for zeolites and the advantages of high activity and anti-deactivation for metal species together, offering a good opportunity to design and preparation of new highly efficient zeolite-based catalysts in the future. Finally, it is suggested perspectives such as rational synthesis of zeolite catalysts by theoretical simulations from the energy comparison, preparation of highly efficient catalysts by incorporating catalytically active sites in zeolite framework from the requirements of catalytic reactions, and green synthesis of zeolites for reduction of harmful gases, polluted water, and solid wastes in industrial processes.

Contents

1 Introduction

2 Adsorption of gaseous reactants in zeolite micropores

2.1 Preparation of zeolite nanocrystals

2.2 Introduction of mesoporosity in zeolite crystals

2.3 Preparation of zeolite nanosheets

3 Conversion of reactants on catalytic sites in zeolites

3.1 Acidic sites in zeolite frameworks

3.2 Heteroatoms in zeolite frameworks

3.3 Multisites in zeolite crystals

4 Desorption of products from zeolite catalysts

4.1 Preparation of zeolite nanocrystals and nanosheets and introduction of mesopores into zeolite crystals

4.2 Adjusting wettability of zeolite catalysts

4.3 Selective adsorption of reaction products by zeolite additives

5 Conclusion and perspectives

Key words

condensed matter / gas-solid phase catalysis / zeolite / catalytic materials

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Fengshou Xiao , Qinming Wu , Chengtao Wang. Condensed Matter Chemistry in Catalysis by Zeolites[J]. Progress in Chemistry. 2023, 35(6): 886-903 https://doi.org/10.7536/PC221008

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Funding

The National Natural Science Foundation of China(U21B20101)

The National Natural Science Foundation of China(22288101)

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References

Funding