Synthetic Strategies of Chemically Stable Metal-Organic Frameworks

Mengrui Yang; Yuxin Xie; Dunru Zhu

doi:10.7536/PC221112

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Prog Chem ›› 2023, Vol. 35 ›› Issue (5) : 683-698. DOI: 10.7536/PC221112

Review

Synthetic Strategies of Chemically Stable Metal-Organic Frameworks

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Abstract

Metal-organic frameworks (MOFs) are a new generation of crystalline porous materials with void space structures constructed from metal ions or clusters and organic ligands through coordination bonds, and have been a hot research topic in the field of coordination chemistry over the past two decades. As the novel multifunctional materials, MOFs have been widely used in various fields due to their high porosities, low densities, large surface areas, tunable pore sizes, diverse topological structures and tailorabilities. Although MOFs have many advantages, most of MOFs materials have relatively lower water and chemical stability and cannot maintain their structures under harsh conditions, which greatly restrict their practical applications under moisture-rich conditions. Therefore, chemically stable MOFs materials will have greater application prospects. In recent years, researchers have carried out a lot of exploration in improving the chemical stability of MOFs, and developed some excellent methods to synthesize chemically stable MOFs. This review will mainly focus on the latest research progress in the syntheses of chemically stable MOFs during the past five years.

Contents

1 Introduction

2 Synthetic strategies of chemically stable MOFs

2.1 Increase the strength of coordination bonds

2.2 Attaching hydrophobic groups onto the linker

2.3 Using pore-partioning ligands for the pore space partition

2.4 Post-synthetic exchange method

2.5 Hydrophobic surface treatment

2.6 Other methods

3 Conclusion and Outlook

Key words

metal-organic frameworks(MOFs) / chemical stability / synthetic strategy

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Mengrui Yang , Yuxin Xie , Dunru Zhu. Synthetic Strategies of Chemically Stable Metal-Organic Frameworks[J]. Progress in Chemistry. 2023, 35(5): 683-698 https://doi.org/10.7536/PC221112

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