Catalytic Mechanism of Oxygen Vacancy Defects in Metal Oxides

Yue Yang; Ke Xu; Xuelu Ma

doi:10.7536/PC221122

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Prog Chem ›› 2023, Vol. 35 ›› Issue (4) : 543-559. DOI: 10.7536/PC221122

Review

Catalytic Mechanism of Oxygen Vacancy Defects in Metal Oxides

Yue Yang ¹ ,
Ke Xu ¹ ,
Xuelu Ma ¹^,²^,^*

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Abstract

Metal oxides have been widely investigated in experimental and industrial catalysis due to their excellent activity, selectivity and stability in many important reactions, especially in some redox reactions, such as CO₂ reduction, water-gas shift (WGS) reaction, reduction of nitrogen, oxygen evolution reaction. It has been proved that metal oxides usually contain many defects, which are the active sites in catalytic reactions, and oxygen vacancies (OVs) are one of the most representative species among them. OVs affect crystal structure and electronic structure of the materials, thus affecting the catalytic activity, so they have great significance to be studied. In this review, we firstly introduce the classification and regulation strategies of OVs based on the formation of them in metal oxides. Secondly, the characteristics and mechanisms of OVs in thermocatalysis, electrocatalysis and photocatalysis were discussed. Finally, the potential applications and future challenges were summarized and prospected.

Key words

oxygen vacancy / metal oxides / mechanism / electronic structure / catalyst design

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Yue Yang , Ke Xu , Xuelu Ma. Catalytic Mechanism of Oxygen Vacancy Defects in Metal Oxides[J]. Progress in Chemistry. 2023, 35(4): 543-559 https://doi.org/10.7536/PC221122

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Funding

Beijing Natural Science Foundation(2232019)

National Natural Science Foundation of China(21902182)

Open Project Program of Fujian Key Laboratory of Functional Marine Sensing Materials(MJUKF-FMSM202202)

Fundamental Research Funds for the Central Universities(2023ZKPYHH01)

Training Program of Innovation and Entrepreneurship for Undergraduates(202203038)

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Received	Revised	Published
2022-11-24	2023-01-04	2023-04-24
Issue Date
2023-02-20

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