Metal Nanocluter Catalysts for Hydrogenation of Carbon Dioxide to Multicarbon Compounds

Yuan Wang; Yulv Yu; Xin Tan

doi:10.7536/PC221235

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Prog Chem ›› 2023, Vol. 35 ›› Issue (6) : 918-927. DOI: 10.7536/PC221235

Review

Metal Nanocluter Catalysts for Hydrogenation of Carbon Dioxide to Multicarbon Compounds

Yuan Wang ¹^,²^,^* ,
Yulv Yu ¹^,² ,
Xin Tan ¹^,²

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Abstract

Selectively catalytic hydrogenation of CO₂ to multi-carbon compounds is of great significance for reducing carbon dioxide emissions and regenerating carbon-containing resources. In this review, we summarize the development of catalytic systems for CO₂ hydrogenation to multi-carbon compounds in recent years. The development of metal nanocluster catalysts for CO₂ hydrogenation to multi-carbon hydrocarbons or alcohols at low temperatures are introduced, and the chemical basis for regulating C₁ and C₂₊ product selectivity in CO₂ hydrogenation is discussed. The progresses in preparing and understanding the structure-function relationship of Pt-Ru bimetallic nanocluster catalysts with the high selectivity for C₂₊ compounds in the CO₂ hydrogenation at low temperatures are discussed. Finally, we elaborate the theory of local charge distribution effect of metal nanocluster catalysts.

Contents

1 Introduction

2 Performance and conversion pathways of CO₂hydrogenation over metal nanocluster catalysts at low temperatures

3 Chemical basis for controlling the product selectivity

4 Preparation and properties of a highly selective PtRu bimetallic nanoclusters catalyst

5 Structural characteristics of active sites of metal nanoclusters

6 Conclusion and perspective

Key words

carbon dioxide / hydrogenation / multi-carbon hydrocarbons / multi-carbon alcohols / Pt-Ru bimetallic nanocluster catalysts / local charge distribution

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Yuan Wang , Yulv Yu , Xin Tan. Metal Nanocluter Catalysts for Hydrogenation of Carbon Dioxide to Multicarbon Compounds[J]. Progress in Chemistry. 2023, 35(6): 918-927 https://doi.org/10.7536/PC221235

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