Condensed Matter Chemistry in Gaseous Molecules Reactions

Ruren Xu; Wenfu Yan

doi:10.7536/PC221236

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Prog Chem ›› 2023, Vol. 35 ›› Issue (6) : 808-820. DOI: 10.7536/PC221236

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Condensed Matter Chemistry in Gaseous Molecules Reactions

Ruren Xu ^* ,
Wenfu Yan

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Abstract

Studying the reactions between gaseous molecules are not only of great significance to promote the development of industry, agriculture and economy, but also play a special role in the construction of condensed chemistry. Under normal conditions, gaseous molecules exist in a dispersed state. Because the stability of the structure of gaseous molecules, in most cases, the reactions between them can only occur under the “activation” of the catalyst with a specific composition and structure. In this paper, we list five simple examples to illustrate that the occurrence, progress and results of gaseous intermolecular reactions are subject to or even completely determined by the characteristics, composition and multi-level structure of the catalysts with specific condensed matter state under reaction conditions. In addition, we also list another reaction route in this paper, that is, under extreme reaction conditions such as high pressure, ultra-low temperature, laser, plasma and supercritical, the electronic and geometric structures and “states” of a few gaseous molecules will change, resulting in the specific condensed matter chemical reactions.

Contents

1 Introduction

2 Catalytic reaetion between gas molecules

Example 1 Homogeneous hydrogenation reaction of olefins

Example 2 Hydrogenation of crotonaldehyde over Co/SiO₂with different surface structures

Example 3 Catalytic dehydrogenation of propane

Example 4 Synthesis reactions of CO/H₂over Ru-containing molten salt catalysts

Example 5 The synthesis of ammonia via reaction of N₂+H₂catalyzed by nitrogenase

3 Condensed matter state reactions between gas molecules under extreme conditions(high pressure)

4 Outlook

Key words

condensed state / gaseous molecules / chemical reaction

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Ruren Xu , Wenfu Yan. Condensed Matter Chemistry in Gaseous Molecules Reactions[J]. Progress in Chemistry. 2023, 35(6): 808-820 https://doi.org/10.7536/PC221236

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Funding

The National Natural Science Foundation of China(22288101)

The National Natural Science Foundation of China(U1967215)

The National Natural Science Foundation of China(21835002)

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Received	Revised	Published
2022-12-09	2023-01-15	2023-06-24
Issue Date
2023-05-18

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