Application of UiO-66 Series MOFs in Proton Exchange Membranes

Mengxin Wang; Xiaocan Zhang; Qiong Zhou

doi:10.7536/PC20250522

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Prog Chem ›› 2025, Vol. 37 ›› Issue (12) : 1731-1757. DOI: 10.7536/PC20250522

Review

Application of UiO-66 Series MOFs in Proton Exchange Membranes

Mengxin Wang ¹^,³ ,
Xiaocan Zhang ²^,³^,^* ,
Qiong Zhou ¹

Author information +

History +

Abstract

Metal-organic frameworks （MOFs） are emerging proton-conducting materials widely used in the modification of proton exchange membranes （PEM）. Among them， the UiO-66 series MOFs （UiO-MOFs） exhibit high thermal and chemical stability， and are easy to synthesize and modify， making them ideal for PEM modification. This paper primarily reviews related research on UiO-MOFs used for PEM modification over the past five years from the perspective of filler design and preparation. Section II introduces the materials and proton conduction mechanisms of UiO-MOFs. Section III summarizes the design of ligands and metal clusters in UiO-MOFs， such as acid/base group modifications and metal cluster replacements. Section IV consolidates the methods for post-synthetic modifications of UiO-MOFs， such as grafting acid/base groups using active functional groups from external crystal structures. Section V presents various composite schemes involving UiO-MOFs and other materials to construct composite fillers with different dimensionalities. Finally， the summary highlights unresolved issues regarding the use of UiO-MOFs in PEMs and proposes future research directions.

Contents

1 Introduction

2 UiO-MOFs and proton conduction mechanism

2.1 UiO-MOFs material properties

2.2 Proton conduction mechanism

3 Design strategy of UiO-MOFs ligands and metal clusters

3.1 Ligand functionalization regulation strategy

3.2 Metal clusters regulation strategy

4 Post-synthetic modification of UiO-MOFs

4.1 Acid group grafting system

4.2 Alkaline group synergistic modification system

5 Construction of UiO-MOFs composite fillers

5.1 Construction strategy of 1D ordered composite fillers

5.2 Construction strategy of 2D composite fillers

5.3 Multi-dimensional control strategy for 3D composite fillers

6 Conclusion and future work

Key words

proton exchange membrane / metal organic frameworks / UiO-66 / proton conduction / composite materials

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Mengxin Wang , Xiaocan Zhang , Qiong Zhou. Application of UiO-66 Series MOFs in Proton Exchange Membranes[J]. Progress in Chemistry. 2025, 37(12): 1731-1757 https://doi.org/10.7536/PC20250522

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Funding

National Natural Science Foundation of China(22105225)

China State Key Laboratory of Heavy Oil Processing Research Fund(CNIF20250204)

Joint Research Institute for Carbon Neutrality(SKLHOP2024115806)

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