Design of Metal-Organic Frameworks Based Photocatalysts and Their Application in Uranium Reduction

Ying Peng; Xiaowen Zhang; Mi Li; Yu Zhang; Yilong Hua; Xiaoyan Wu

doi:10.7536/PC20251108

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Prog Chem ›› 2026, Vol. 38 ›› Issue (5) : 832-848. DOI: 10.7536/PC20251108

Review

Design of Metal-Organic Frameworks Based Photocatalysts and Their Application in Uranium Reduction

Ying Peng ¹ ,
Xiaowen Zhang ¹^,²^,^* ,
Mi Li ¹^,² ,
Yu Zhang ¹^,² ,
Yilong Hua ¹^,² ,
Xiaoyan Wu ¹^,²

Author information +

History +

Abstract

The photocatalytic reduction of uranium can utilize sunlight， and convert soluble U（VI） into recyclable solid substances， thereby solving the two major problems of radioactive wastewater treatment and seawater uranium extraction. Metal-organic frameworks （MOFs）， a new type of functional porous three-dimensional （3D） crystalline materials， have large specific surface area， special metal clusters， designable organic ligands， adjustable unique morphology and pore structure， hence attracted extensive attention in the fields of photocatalysis and photochemistry. This review summarizes the design strategies for optimizing the performance of MOFs-based photocatalysts， probes into the mechanism of photocatalytic U（VI） reduction by MOFs， and elaborates on the application of MOFs in photocatalytic U（VI） reduction. Finally， the current challenges of MOFs photocatalysts in the application of U（VI） reduction are discussed， and a forward-looking perspective on the future research directions are proposed.

Contents

1 Introduction

2 Design of MOFs-based photocatalysts

2.1 Optimization of MOFs structure

2.2 Synthesis of MOFs composites

2.3 Synthesis of MOFs derivatives

3 Application of MOFs-based photocatalysts in U（Ⅵ） reduction

3.1 Mechanism of photocatalytic U（Ⅵ） reduction

3.2 Design directions of MOFs-based photocatalysts

3.3 Performances of different MOFs-based photo-catalysts for U（Ⅵ） reduction

4 Conclusion and outlook

Key words

metal-organic frameworks / photocatalysis / uranium reduction / mechanism

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Ying Peng , Xiaowen Zhang , Mi Li , et al . Design of Metal-Organic Frameworks Based Photocatalysts and Their Application in Uranium Reduction[J]. Progress in Chemistry. 2026, 38(5): 832-848 https://doi.org/10.7536/PC20251108

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Funding

National Natural Science Foundation of China(52374173)

Hunan Provincial Natural Science Foundation of China(2025JJ50255)

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