Low-Temperature Electrooxidation Catalysts for Methane Conversion

Shiyu Jiang, Jiaxin Jiang, Haosen Xiong, Shuyong Shang, Ge He, Qiang Zhang

Prog Chem ›› 2026, Vol. 38 ›› Issue (3) : 421-442.

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Prog Chem ›› 2026, Vol. 38 ›› Issue (3) : 421-442. DOI: 10.7536/PC20251117
Review

Low-Temperature Electrooxidation Catalysts for Methane Conversion

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Abstract

This article reviews the challenges and recent advancements in the utilization of methane （CH4） resources via low-temperature electrochemical oxidation （CH4OR） for producing value-added chemicals. Conventional indirect pathways， including methane reforming， are energy-intensive and operate under harsh conditions. In contrast， thermal catalytic partial oxidation frequently results in over-oxidation， thereby limiting its practical applications. In contrast， electrochemical CH4OR represents a promising alternative， facilitating efficient methane conversion under mild conditions， compatible with renewable energy sources， and providing advantages in product separation and transport. This review explores the mechanistic aspects of C—H bond activation during CH4OR， encompassing both direct and radical-mediated indirect pathways.

Contents

1 Introduction

2 The mechanism of low-temperature electrooxidation of methane

2.1 Direct activation mechanism of methane dehydrogenation

2.2 Mechanism of methane dehydrogenation activated by reactive oxygen species

2.3 Kinetic and thermodynamic control in the CH4OR

3 Methane electrooxidation catalyst

3.1 Noble metal catalysts

3.2 Alloy catalysts

3.3 Transition metal oxide catalysts

3.4 MOFs catalysts

3.5 Single atom catalysts

4 Defect engineering： material design strategy for catalytic performance optimization

5 Conclusions and prospects

Key words

methane electrooxidation / oxygen-containing compounds / reaction mechanism / catalyst

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Shiyu Jiang , Jiaxin Jiang , Haosen Xiong , et al . Low-Temperature Electrooxidation Catalysts for Methane Conversion[J]. Progress in Chemistry. 2026, 38(3): 421-442 https://doi.org/10.7536/PC20251117

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Funding

National Natural Science Foundation of China(21902017)
China Postdoctoral Science Foundation(2024M753166)
Natural Science Foundation of Chongqing of China(CSTB2025NSCQ-GPX0960)
Natural Science Foundation of Chongqing of China(CSTB2025TIAD-KPX0017)
Science and Technology Research Program of Chongqing municipal Education Commission of China(KJQN202301121)
Natural Science Foundation of Sichuan of China(2024NSFSC0295)
Natural Science Foundation of Sichuan of China(2024ZYD0157)
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