Nano-State Layered Double Hydroxides Based Materials for Photo-Driven C1 Chemical Conversion

Chi Duan; Zhenhua Li; Tierui Zhang

doi:10.7536/PC221216

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Prog Chem ›› 2023, Vol. 35 ›› Issue (6) : 940-953. DOI: 10.7536/PC221216

Review

Nano-State Layered Double Hydroxides Based Materials for Photo-Driven C₁ Chemical Conversion

Chi Duan ¹ ,
Zhenhua Li ¹^,^* ,
Tierui Zhang ¹^,²^,^*

Author information +

History +

Abstract

Energy is the basic guarantee for human survival. As an important reaction in field of energy, C₁ chemical conversion has safeguarded the development of human society. With the proposal of "double carbon" goal, energy saving-emission reduction and environmental friendliness have been the new pursuit of C₁ catalytic conversion researchers. Recently, photo-driven C₁ chemical conversion has attracted researchers’ attention through which C₁ small molecules can be transformed into various value-added products under ambient condition. Layered double hydroxides (LDH) have gained wide application in photo-driven C₁ chemical conversion for their distinctive two-dimensional layered structure. Herein, we review the latest progress achieved in nano-state LDH based materials for photo-driven C₁ chemical conversion from three aspects containing LDH precursors acting as catalyst, LDH derivatives acting as catalyst and LDH acting as catalyst carrier, and conclude the challenges this field may face in the future. Through analyzing and discussing above-mentioned work, we hope to offer researchers some inspiration on photo-driven C₁ chemistry.

Contents

1 Introduction

2 A brief introduction of LDH

2.1 Structural composition of LDH

2.2 Basic properties of LDH

3 Application of LDH based materials in photo-driven C₁conversion

3.1 LDH precursors as catalyst

3.2 LDH derivatives as catalyst

3.3 LDH as catalyst carrier

4 Conclusion and outlook

Key words

C₁ chemical conversion / LDH / photo-driven / valve-added chemicals

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Chi Duan , Zhenhua Li , Tierui Zhang. Nano-State Layered Double Hydroxides Based Materials for Photo-Driven C₁ Chemical Conversion[J]. Progress in Chemistry. 2023, 35(6): 940-953 https://doi.org/10.7536/PC221216

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Funding

The National Natural Science Foundation of China(51825205)

The National Natural Science Foundation of China(52120105002)

The National Natural Science Foundation of China(22088102)

The National Natural Science Foundation of China(22209190)

The Postdoctoral Science Foundation of China(2021M703288)

The Postdoctoral Science Foundation of China(2022T150665)

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Received	Revised	Published
2022-12-28	2023-05-19	2023-06-24
Issue Date
2023-05-25

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