Photocatalytic Production of Hydrogen Peroxide from Covalent Organic Framework Materials

Anqi Chen; Zhiwei Jiang; Juntao Tang; Guipeng Yu

doi:10.7536/PC230724

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Prog Chem ›› 2024, Vol. 36 ›› Issue (3) : 357-366. DOI: 10.7536/PC230724

Review

Photocatalytic Production of Hydrogen Peroxide from Covalent Organic Framework Materials

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Abstract

Hydrogen peroxide (H₂O₂) is an important green oxidizing agent, but the main anthraquinone process for production thereof suffers high energy consumption and large safety risks. Artificial photosynthesis H₂O₂from water and oxygen features safe, environmentally friendly and energy-saving characteristics and has gradually become a research focus. Covalent organic frameworks (COFs) have been widely used in the photocatalytic production of H₂O₂ for their high specific surface area, good photocatalytic performance and structural tunability. This review summarizes the recent research progress in the field of COFs photocatalytic production of H₂O₂, discussing the reaction mechanisms for the production of H₂O₂ through oxygen reduction, water oxidation, and dual-channel processes. It introduces methods to improve the photocatalytic production of H₂O₂ by regulating the optical bandgap, enhancing charge separation capability, and improving carrier mobility of COFs through structural design and functional group modification. These methods contribute to the design of efficient, stable, and sustainable COFs for photocatalytic production of H₂O₂.

Contents

1 Introduction

2 Hydrogen peroxide production by ORR pathway

2.1 Direct one-step two-electron oxygen reduction mechanism

2.2 Indirect two-step single-electron oxygen reduction mechanism

3 Hydrogen peroxide production by WOR pathway

4 Dual-channel path production of hydrogen peroxide

5 Conclusion and outlook

Key words

covalent organic framework / hydrogen peroxide / photocatalysis / oxygen reduction / water oxidation

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Anqi Chen , Zhiwei Jiang , Juntao Tang , et al. Photocatalytic Production of Hydrogen Peroxide from Covalent Organic Framework Materials[J]. Progress in Chemistry. 2024, 36(3): 357-366 https://doi.org/10.7536/PC230724

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