MOFs-Based Photoelectrochemical Sensing Interface and Its Applications

Cunyin Zhou; Juan Huang; Qiong Wang; Hao Tang; Yunchu Hu; Wenlei Wang

doi:10.7536/PC230913

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Prog Chem ›› 2024, Vol. 36 ›› Issue (6) : 893-903. DOI: 10.7536/PC230913

Review

MOFs-Based Photoelectrochemical Sensing Interface and Its Applications

Cunyin Zhou ¹ ,
Juan Huang ¹ ,
Qiong Wang ¹^,²^,^* ,
Hao Tang ² ,
Yunchu Hu ¹ ,
Wenlei Wang ¹

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Abstract

photoelectrochemical sensing analysis is a rapidly developing new analytical technology in recent years,and photoelectric active materials are The key to photoelectrochemical sensing detection.metal-organic frameworks(MOFs)and their derivatives may be ideal carriers for the construction of photoelectrochemical sensing interfaces by dispersing photoelectrically active substances.Due to the"antenna effect"of organic ligands in MOFs,the metal clusters can be regarded as activated discrete semiconductor quantum dots,giving them photoelectric properties similar to those of semiconductors.the modification of MOFs materials with carbon-based compounds,organic polymers,noble metal nanoparticles,inorganic oxides,and quantum dots,and the construction of MOFs-based photoelectrochemical sensing interfaces,can improve the electrical conductivity of MOFs,promote the separation of photogenerated electrons-holes,and thus improve the photoelectric conversion efficiency.the MOFs-based photoelectrochemical sensing interfaces amplify the signal generated by photoelectrochemical sensing,enabling ultra-sensitive detection of the target object.based on these,this study provides a detailed introduction to the photoelectric activity mechanism,synthesis methods,and strategies for constructing photoelectric activity interfaces of MOFs-based materials.the applications of MOFs-based materials in photoelectrochemical sensing detection of small molecule compounds,immunoassay,enzyme activity and environmental analysis in recent years have been comprehensively reviewed.Finally,current challenges and future perspectives in this field are also proposed.

Contents

1 Introduction

2 MOFs-based photoelectric active materials

2.1 Photoelectric activity mechanism

2.2 Synthesis of MOFs-based photoelectric active materials

3 Strategies for the construction of MOFs-based photoelectrochemical sensing interfaces

3.1 MOFs-based photoelectrochemical sensing interfaces constructed by carbon-based compound modification

3.2 MOFs-based photoelectrochemical sensing interfaces constructed by organic polymer modification

3.3 MOFs-based photoelectrochemical sensing interfaces constructed by noble metal nanoparticle modification

3.4 MOFs-based photoelectrochemical sensing interfaces constructed by inorganic oxide modification

3.5 MOFs-based photoelectrochemical sensing interfaces constructed by quantum dots modification

4 MOFs-based photoelectrochemical sensing interfaces for analytical testing applications

4.1 Application of MOFs-based photoelectrochemical sensing interfaces for small molecule detection

4.2 Application of MOFs-based photoelectrochemical sensing interfaces for immunoassay detection

4.3 Application of MOFs-based photoelectrochemical sensing interfaces for enzyme analysis detection

4.4 Application of MOFs-based photoelectrochemical sensing interfaces for protein analysis detection

4.5 Application of MOFs-based photoelectrochemical sensing interfaces for environmental analysis detection

5 Conclusion and outlook

Key words

MOFs-based materials / photoelectrochemical sensing interface / photoelectrochemical sensing analysis

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Cunyin Zhou , Juan Huang , Qiong Wang , et al . MOFs-Based Photoelectrochemical Sensing Interface and Its Applications[J]. Progress in Chemistry. 2024, 36(6): 893-903 https://doi.org/10.7536/PC230913

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Funding

National Natural Science Foundation of China(41977129)

Hunan Provincial Natural Science Foundation of China(2022JJ90020)

Excellent Youth Funding of Hunan Provincial Education Department of China(22B0246)

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Received	Revised	Published
2023-09-26	2024-02-28	2024-06-24
Issue Date
2024-04-16

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