Application of Two-Dimensional Catalysts in Selective Oxidation of Methane

Yuyang Sun; Wenxi Wang; Wencui Li; Hanying Qin; Jiaxin Cai; Zhen Zhao

doi:10.7536/PC241206

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Prog Chem ›› 2025, Vol. 37 ›› Issue (8) : 1218-1234. DOI: 10.7536/PC241206

Review

Application of Two-Dimensional Catalysts in Selective Oxidation of Methane

Yuyang Sun ¹ ,
Wenxi Wang ¹ ,
Wencui Li ¹^,^* ,
Hanying Qin ² ,
Jiaxin Cai ² ,
Zhen Zhao ¹^,²^,^*

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History +

Abstract

Two-dimensional materials，with their high specific surface areas and tunable electronic structures，have shown significant advantages in the enhancement of catalytic efficiency，selectivity，and stability. Their ability to catalyze the conversion of methane into high-value chemicals is of great importance for sustainable energy utilization and environmental protection. This paper reviews the progress of the application of two-dimensional materials in the low-temperature selective oxidation of methane，summarizes the two mechanisms of C—H bond fracture during methane oxidation and lists several typical two-dimensional materials （such as graphene，transition metal sulfides，MXenes，MOFs，metal oxides and their synthesis methods. This paper focuses on investigating the catalytic performance of these materials doped with metal active sites for the selective oxidation of methane using different oxidants （such as H₂O₂，H₂+O₂，O₂，and CO+O₂），emphasizing the role of two-dimensional materials in the regulation of active sites and optimization of reaction pathways. Finally，the potential，challenges and future development direction of two-dimensional materials in solving the problem of methane activation and promoting the progress of energy technology are prospected.

Contents

1 Introduction

2 Overview of two-dimensional material catalysts

2.1 Graphene

2.2 Transition metal chalcogenides

2.3 Mxenes

2.4 MOFs

2.5 Metal oxides

2.6 Other materials

3 Mechanism of C—H bond cleavage of methane oxidation

3.1 Radical mechanism

3.2 M-C σ-bond mechanism

4 The application of two-dimensional materials doped metal atom catalysts in methane oxidation reaction

4.1 Precious metals

4.2 Non-precious metals

4.3 Two-dimensional materials doped with metal atom catalysts

5 Conclusion and outlook

Key words

methane conversion / two-dimensional materials / heterogeneous catalysis / C—H bond activation / selective oxidation

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Yuyang Sun , Wenxi Wang , Wencui Li , et al . Application of Two-Dimensional Catalysts in Selective Oxidation of Methane[J]. Progress in Chemistry. 2025, 37(8): 1218-1234 https://doi.org/10.7536/PC241206

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Funding

the National Natural Science Foundation of China(22402131)

the National Natural Science Foundation of China(92145301)

the National Natural Science Foundation of China(91845201)

the Fundamental Research Funds for the Liaoning Universities(42400502105)

Doctoral Research Initiation Project of Liaoning Province(2025-BS-0792)

Doctoral Research Initiation Project of Liaoning Province(2025-BS-0970)

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