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Abbreviation (ISO4): Prog Chem      Editor in chief: Jincai ZHAO

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Preparation of Heteroatom Doped Graphene and Its Application as Electrode Materials for Supercapacitors
Yunpeng Wu, Xiaofeng Wang, Benxian Li, Xudong Zhao, Xiaoyang Liu
Prog Chem, 2023, 35(7): 1005-1017.   DOI: 10.7536/PC220811

Material Atom(s) Synthesis method/ React condition Dopant Carbon source Performance Ref
1 N-HtrGO N Hydrothermal/150℃, 12 h Urea GO 244 F/g at 50 mV/s, 105% at 2000 cycles 86
2 NHGNSs N Thermally annealed/ 360℃, 5 h NH3 GO 126 F/g at 1 A/g, 91% at 2000 cycles 66
3 PG-Ni N Thermally annealed/ 800℃, 2 h N2 GO 575 F/g at 0.5 A/g, 89.5% at 10 000 cycles 68
4 FNG N Ball milling/500 rpm, 24 h Melamine Expanded graphite 83.8 mF/cm2 at 0.6 mA/cm2, 93.8% at 5000 cycles 38
5 NG-DWCNT N CVD/ 1300℃ under Ar Urea Ethanol 563 F/g at 50 A/g, 94.35% at 5000 cycles 27
6 NGH N Hydrothermal/ 90℃, 4 h Carbamide GO 199.8 F/g at 2 A/g, 97% at 20000 cycles 87
7 NG N Hydrogel strategy Pyrrole GO 455.4 F/g at 1 A/g, 97.4% at 5000 cycles 88
8 BMG B Hydrothermal/180℃, 4 h Boric acid GO 336 F/g at 0.1 A/g, 98% at 5000 cycles 89
9 HTBAGO B Supercritical fluid processing/400℃, 1 h Boric acid GO 286 F/g at 1 A/g, 96% at 10 000 cycles 70
10 B-rGO B Electrochemical synthesis Boric acid GO 446 F/g at 0.1 A/g, 95.6% at 2000 cycles 90
11 BGNS B Solvothermal/150℃, 12 h Boric acid GO 125 F/g at 1 A/g, 83% at 2000 cycles 91
12 P-TRG P Thermal annealing/ 800℃, 30 min H3PO4 GO 115 F/g at 0.05 A/g, 97% at 5000 cycles 72
13 PO-graphene P Electrochemical synthesis (NH4)3PO4 Graphite rod 1634.2 F/g at 3.5 mA/cm2, 67% at 500 cycles 92
14 PGA P Solvothermal/150℃, overnight Phytic Acid GO 225.3 F/g at 1 A/g, 95% at 10 000 cycles 73
15 PGO P Supercritical fluid processing/400℃, 1 h Na3PO4 GO 518 F/g at 1 A/g, 98% at 5000 cycles 93
16 S-GEs S Electrochemical synthesis H2SO4 Pencil graphite 1833 mF/cm2 at 10 mA/cm2, 95% at 1000 cycles 74
17 S@G S Heat treatment/155℃, 8 h S Nanomesh graphene 257 F/g at 0.25 A/g, 87% at 10 000 cycles 94
18 S-rGO S Microwave-assisted synthesis/140℃, 30 min Na2S GO 237.6 F/g at 0.1 A/g, 113% at 5000 cycles 75
19 L-P LIG S Laser direct writing Polyethersulfone Lignin 22 mF/cm2 at 0.05 mA/cm2, 89.8% at 9000 cycles 95
20 Cl-RGOFs Cl Hydrothermal/180℃, 3 h HCl GO 210 F/g at 1 A/g, 94.3% at 5000 cycles 77
21 FGA F Hydrothermal/150℃, 12 h HF GO 279.8 F/g at 0.5 A/g, 94.3% at 5000 cycles 96
22 NiNOG Ni, N, O Ball milling/ 400 rpm, 10 h Ni(NO3)2·6H2O Melamine Graphite 532 F/g at 1 A/g, 87.5% at 10 000 cycles 40
23 NP-rGO N, P Supramolecular
polymerization		 Melamine
Phytic acid		 GO 416 F/g at 1 A/g, 94.63% at 10 000 cycles 97
24 s-SPG S, P Thermal activation/ 900℃, 1 h Phytic acid
Thioglycolic acid		 GO 168 F/g at 1 A/g, 91.7% at 2000 cycles 54
25 N, S, PHHGO N, S, P Hydrothermal/ 140℃, 2 h NH4H2PO4
L-cysteine		 GO 295 F/g at 1 A/g, 93.5% at 10 000 cycles 85
26 S, N-FLG N, S Microwave irradiation/900 W and 2.45 GHz for a few seconds H2SO4 HNO3 Graphite 298 F/g at 1 A/g, 95% at 10 000 cycles 84
Table 1 Performance of heteroatom-doped graphene as electrode materials for supercapacitors
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